Synonyms for tighten
verb
To make tight
compress, condense, squeeze, bind, contract, strangle, constrict, crush, cramp, pinch, grip more tightly, clench, screw down, add pressure; see also stretch 2.
Antonyms loosen*, relax, unloose.
To become tight
contract, harden, congeal, stiffen, toughen, become more disciplined, become stricter.
Antonyms melt, soften*, liquefy.
See tighten in Webster's New World Roget's A-Z Thesaurus II
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